Moore grew up in Southern California's San Fernando Valley and attended Hale Junior High School in Woodland Hills, where he met the other members of Fishbone's original lineup. Moore's father played saxophone for Count Basie, and his parents exposed him to jazz, soul and funk music. He then attended El Camino Real High School in Woodland Hills.
In addition to his regular duties with Fishbone, in 1993 Moore released a poetry anthology titled Dr. Madd Vibe's Comprehensive Linkology. In 1997 he released his first solo CD, also titled Dr. Madd Vibe's Comprehensive Linkology, as well as his first video titled The Delusional Quandaries Of Dr. Madd Vibe. In 2000 Moore released another CD/video set titled The Yin-Yang Thang, and in 2006 he released the CD Dr. Madd Vibe's Medicine Cabinet. Moore also made a cameo appearance as the bandleader in the movie Idlewild, featuring Outkast members Big Boi and Andre 3000. On June 26, 2012, Angelo Moore and the Rondo Brothers released the single "Brand New Step" under Ninth Street Opus record label.
Moore in July 2021 played the role of Manager in the music video for "Holier than Thou", a Metallica cover song by Off!.

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