Grisetti was born in Washington, D.C. and grew up outside of Roanoke, Virginia. He attended high school at the North Carolina School of the Arts to graduate in 2000 with a diploma in Drama. He attended college at The Boston Conservatory where he graduated in 2004 with a Bachelor of Fine Arts in Musical Theatre.
Grisetti starred in the York Theatre's 2008-2009 musical adaption of Enter Laughing (originally titled So Long, 174th Street), garnering a Theatre World Award for "Outstanding Debut Performance" as well as Drama Desk, Outer Critics Circle, Lucille Lortel and Drama League Award nominations. Grisetti was supposed to have made his Broadway debut in the 2009–2010 season, starring as "Eugene Morris Jerome" in the Neil Simon revival of Broadway Bound, directed by David Cromer. Because of poor ticket sales, Broadway Bound's sister show (Brighton Beach Memoirs) closed just days after opening at the Nederlander Theatre, canceling Broadway Bound two weeks before its scheduled premiere.
Grisetti's actual Broadway debut took place in the original musical It Shoulda Been You in 2015, playing the role of Marty Kaufman. He received nominations from the Drama Desk Awards and the Outer Critics Circle for his performance, and won one of two 2015 Clarence Derwent Awards. He returned to Broadway in 2016 to replace John Cariani as Nigel Bottom in "Something Rotten!"

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