Liboiron was born the youngest of three boys in a small farming community in Jenner, Alberta, where he and his two older brothers were raised. He is the son of Lorraine Mack and Marcel Liboiron. His mother, an artist, supportive of his desire to act, once drove her son to Vancouver for acting classes and auditions.
Liboiron was cast in TV films before his breakout role in the Canadian teen drama television series Degrassi: The Next Generation. In 2011, Liboiron played Josh Shannon in the sci-fi television series Terra Nova, the son of the lead character, played by Jason O'Mara, and his wife, played by Shelley Conn.
In 2013, Liboiron was cast in a lead role opposite Bill Skarsgård and Famke Janssen as high school student and Romani werewolf Peter Rumancek in the Netflix original series Hemlock Grove. Liboiron reprised his role in the second and third season of the series.

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