Buchheim was born in Weimar, in the Grand Duchy of Saxe-Weimar-Eisenach (present-day Thuringia), the second son of artist Charlotte Buchheim. She was unmarried, and he was raised by his mother and her parents. They lived in Weimar until 1924, then Rochlitz until 1932, and finally Chemnitz. He began contributing to newspapers in his teens and put on an exhibition of his drawings in 1933, when he was 15.
He travelled to the Baltic Sea with his brother, and canoed along the Danube to the Black Sea. After taking his Abitur in 1937, he spent time in Italy, where he wrote his first book, Tage und Nächte steigen aus dem Strom. Eine Donaufahrt ("Days and nights rise from the river. A journey on the Danube"), published in 1941. He studied art in Dresden and Munich in 1939, and volunteered for the Kriegsmarine in 1940.
Buchheim was a Sonderführer in a propaganda unit of the Kriegsmarine in the Second World War, writing as a war correspondent about his experiences on minesweepers, destroyers and submarines. He also made drawings and took photographs.

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