Gunn was born in St. Louis, Missouri. He was the son of Mary and George Gunn, a laborer, and was one of seven siblings. After his mother died, his family separated. Moses left home and rode the railroad at just 12 years old. He returned to St. Louis and attended school while living at the home of Jewel Richie, his English teacher.
He graduated from Tennessee State University, where he became a member of Omega Psi Phi fraternity Rho Psi chapter. After serving in the United States Army, he attended graduate school at the University of Kansas, earning a master's degree. He taught briefly at Grambling College before attempting an acting career in New York City.
A character actor of film and television, Gunn also enjoyed a successful career on stage. He made his New York City stage debut in the original off-Broadway production of Jean Genet's The Blacks (1962). He performed many Shakespearean roles in Joseph Papp's Shakespeare in the Park, winning an Obie Award for his portrayal of Aaron in Titus Andronicus.

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