Damon was born in Brooklyn, New York, the son of Marvin Leonard Zonis, who was a manufacturer. Damon's parents were Russian Jewish immigrants who made their home in America after fleeing the Bolshevik Revolution.
After a series of roles on Broadway, Damon's appearance as the Prince in the 1965 version of Rodgers and Hammerstein's Cinderella starring Lesley Ann Warren helped pave the way to a long career in television soap opera. That same year, he had a prominent featured role in the Broadway musical Do I Hear a Waltz? written by Richard Rodgers (music) and Stephen Sondheim (lyrics). He had earlier appeared in an Off-Broadway revival of The Boys From Syracuse with music by Rodgers and lyrics by Lorenz Hart. Damon is prominently featured on the cast albums of these musicals, as well as the hit Irma La Douce (1960).
Moving to Great Britain, Damon starred in the hit West End musical Charlie Girl with Anna Neagle in 1965, and was selected to appear as American secret agent Craig Stirling, alongside British actors Alexandra Bastedo and William Gaunt, in the ITC series The Champions. He also appeared with Roger Moore in an episode of The Saint which has been credited as the inspiration for the later series The Persuaders!, with Damon's role being played by Tony Curtis. In 1968, he appeared in the BBC TV adaptation of The £1,000,000 Bank Note and played Henry Adams in the starring role. Damon also played magician Harry Houdini in a lavishly staged London musical, Man of Magic. In 1970 Damon released an LP called Stuart 'Champion' Damon recorded on Reflection records REF L7 which failed to chart.

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